Tuning of the Interconnecting Layer for Monolithic Perovskite/ Organic Tandem Solar Cells with Record Efficiency Exceeding 21%

Pang Wang, Wei Li, Oskar J. Sandberg, Chuanhang Guo, Rui Sun, Hui Wang, Donghui Li, Huijun Zhang, Shili Cheng, Dan Liu, Jie Min, Ardalan Armin, and Tao Wang

Nano Lett. 2021, 21, 18, 7845–7854

Publication Date:September 10, 2021

https://doi.org/10.1021/acs.nanolett.1c02897

In this paper the researchers utilize the wide-bandgap CsPbI2Br semiconductor and narrow-bandgap PM6:Y6-BO blend to fabricate perovskite/organic tandem solar cells with an efficiency of 21.1% and a very small tandem open-circuit voltage loss of 0.06 V.

The photon absorption rate distribution of polyTPD and PBDB-T-Si based TSCs were simulated using the transfer-matrix model via SETFOS (version number: SETFOS 5.1)

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The Optical Origin of Near-Unity External Quantum Efficiencies in Perovskite Solar Cells

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Fluorinated Oligomer Wrapped Perovskite Crystals for Inverted MAPbI 3 Solar Cells with 21% Efficiency and Enhanced Stability